Find in Library
Search millions of books, articles, and more
Indexed Open Access Databases
Comparison of different Aethalometer correction schemes and a reference multi-wavelength absorption technique for ambient aerosol data
oleh: J. Saturno, C. Pöhlker, D. Massabò, J. Brito, S. Carbone, Y. Cheng, X. Chi, F. Ditas, I. Hrabě de Angelis, D. Morán-Zuloaga, M. L. Pöhlker, L. V. Rizzo, D. Walter, Q. Wang, P. Artaxo, P. Prati, M. O. Andreae, M. O. Andreae, M. O. Andreae
Format: | Article |
---|---|
Diterbitkan: | Copernicus Publications 2017-08-01 |
Deskripsi
Deriving absorption coefficients from Aethalometer attenuation data requires different corrections to compensate for artifacts related to filter-loading effects, scattering by filter fibers, and scattering by aerosol particles. In this study, two different correction schemes were applied to seven-wavelength Aethalometer data, using multi-angle absorption photometer (MAAP) data as a reference absorption measurement at 637 nm. The compensation algorithms were compared to five-wavelength offline absorption measurements obtained with a multi-wavelength absorbance analyzer (MWAA), which serves as a multiple-wavelength reference measurement. The online measurements took place in the Amazon rainforest, from the wet-to-dry transition season to the dry season (June–September 2014). The mean absorption coefficient (at 637 nm) during this period was 1.8 ± 2.1 Mm<sup>−1</sup>, with a maximum of 15.9 Mm<sup>−1</sup>. Under these conditions, the filter-loading compensation was negligible. One of the correction schemes was found to artificially increase the short-wavelength absorption coefficients. It was found that accounting for the aerosol optical properties in the scattering compensation significantly affects the absorption Ångström exponent (<i>å</i><sub>ABS</sub>) retrievals. Proper Aethalometer data compensation schemes are crucial to retrieve the correct <i>å</i><sub>ABS</sub>, which is commonly implemented in brown carbon contribution calculations. Additionally, we found that the wavelength dependence of uncompensated Aethalometer attenuation data significantly correlates with the <i>å</i><sub>ABS</sub> retrieved from offline MWAA measurements.