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In this work, the asymmetrical rolling of 860 μm thick high-purity titanium (HP-Ti) strips is investigated. HP-Ti ultra-thin strips are produced in thicknesses ranging from 280 μm to 20 μm. The microstructure and texture evolution of HP-Ti ultra-thin strips were analyzed using electron backscattering diffraction (EBSD), transmission electron microscopy (TEM), and X-ray diffraction (XRD). The raw strips have a homogeneous and equiaxed microstructure, containing some face-centered cubic (FCC) Ti laths. With a rise in rolling reduction, equiaxed grains change into deformation structures characterized by a high density of dislocations. The formation of an ultra-fine grained microstructure and the elimination of FCC-Ti laths come next. The influence of grain rotation and slip systems on the development of texture in ultra-thin strips during rolling reduction is illustrated through the analysis of {0002} pole figures and orientation distribution function. The tensile qualities of ultra-thin strips are correlated with their microstructure.