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For continuous sliding mode control (SMC) in the unified chaotic systems subjected to matched/unmatched uncertainties, a novel chattering-free SMC design is proposed. First, an augmented state is introduced such that it becomes possible to develop a continuous controller to eliminate the undesired chattering which often appears in the typical SMC. Then by using this chattering-free controller, the chaos behavior in unified chaotic systems with matched uncertainties can be completely suppressed. As for the unmatched uncertainties, every state of controlled systems can be driven and limited to a predictable bound, which is not addressed in the literature. Finally, the effectiveness of the proposed chattering-free controller is verified by the numerical simulations.