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Graphene nanoplatelet (GNP)–epoxy composites were fabricated for the investigation of the dielectric permittivity and microwave absorption in a frequency range from 8 to 20 GHz. The intrinsically conductive GNP particles and polarized interfacial centers in the composites contribute to the microwave absorption. A minimum reflection loss of −14.5 dB at 18.9 GHz is observed for the GNP–epoxy composites with 15 wt. % GNP loading, which is mainly attributed to electric conductivity and the charge multipoles at the polarized interfaces in the GNP–epoxy composites.