Enhanced electron–phonon scattering in Janus MoSSe

oleh: Rong Guo, Xiangtian Bu, Shudong Wang, Guojun Zhao

Format: Article
Diterbitkan: IOP Publishing 2019-01-01

Deskripsi

Electron–phonon (e–ph) interaction in monolayer Janus MoSSe has been investigated using ab initio approach. We find that the asymmetric structure induced net dipole moment in MoSSe introduce an enhanced e–ph interaction compared to the symmetric MoS _2 . Through the mode resolved scattering analysis, we demonstrate that the out-of-plane optical mode in MoSSe contributing to the total e–ph scattering rates are much more than MoS _2 . Around the band edges, the maximum mean free paths (MFPs) of both electrons and holes along zigzag (ZZ) direction are found to be 4 nm in MoSSe, while the MFPs along armchair directions are significantly shorter than along ZZ direction, meaning the highly anisotropic transport properties in MoSSe.