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The optimal auxiliary function method (OAFM) is introduced and used in the analysis of a nonlinear system containing coupled Schrödinger–KdV equations, all within the framework of the Caputo operator. The OAFM, known for its efficiency in solving nonlinear issues, is used to obtain approximate solutions for the coupled equations’ complicated dynamics. Numerical and graphical assessments prove the suggested method’s correctness and efficiency. This study contributes to the understanding and analysis of coupled Schrödinger–KdV equations and their many applications by providing insights into the behavior of nonlinear systems within mathematical physics.