Decreased Anthropogenic CO<sub>2</sub> Emissions during the COVID-19 Pandemic Estimated from FTS and MAX-DOAS Measurements at Urban Beijing

oleh: Zhaonan Cai, Ke Che, Yi Liu, Dongxu Yang, Cheng Liu, Xu Yue

Format: Article
Diterbitkan: MDPI AG 2021-02-01

Deskripsi

The COVID-19 pandemic has led to ongoing reductions in economic activity and anthropogenic emissions. Beijing was particular badly affected by lockdown measures during the early months of the COVID-19 pandemic. It has significantly reduced the CO<sub>2</sub> emission and toxic air pollution (CO and NO<sub>2</sub>). We use column-averaged dry-air mole fractions of CO<sub>2</sub> and CO (XCO<sub>2</sub> and XCO) observed by a ground-based EM27/SUN Fourier transform spectrometer (FTS), the tropospheric NO<sub>2</sub> column observed by MAX-DOAS and satellite remote sensing data (GOSAT and TROPOMI) to investigate the variations in anthropogenic CO<sub>2</sub> emission related to COVID-19 lockdown in Beijing. The anomalies describe the spatio-temporal enhancement of gas concentration, which relates to the emission. Anomalies in XCO<sub>2</sub> and XCO, and XNO<sub>2</sub> (ΔXCO<sub>2</sub>, ΔXCO, and ΔXNO<sub>2</sub>) for ground-based measurements were calculated from the diurnal variability. Highly correlated daily XCO and XCO<sub>2</sub> anomalies derived from FTS time series data provide the ΔXCO to ΔXCO<sub>2</sub> ratio (the correlation slope). The ΔXCO to ΔXCO<sub>2</sub> ratio in Beijing was lower in 2020 (8.2 ppb/ppm) than in 2019 (9.6 ppb/ppm). The ΔXCO to ΔXCO<sub>2</sub> ratio originating from a polluted area was significantly lower in 2020. The reduction in anthropogenic CO<sub>2</sub> emission was estimated to be 14.2% using FTS data. A comparable value reflecting the slowdown in growth of atmospheric CO<sub>2</sub> over the same time period was estimated to be 15% in Beijing from the XCO<sub>2</sub> anomaly from GOSAT, which was derived from the difference between the target area and the background area. The XCO anomaly from TROPOMI is reduced by 8.7% in 2020 compared with 2019, which is much smaller than the reduction in surface air pollution data (17%). Ground-based NO<sub>2</sub> observation provides a 21.6% decline in NO<sub>2</sub>. The NO<sub>2</sub> to CO<sub>2</sub> correlation indicates a 38.2% decline in the CO<sub>2</sub> traffic emission sector. Overall, the reduction in anthropogenic CO<sub>2</sub> emission relating to COVID-19 lockdown in Beijing can be detected by the Bruker EM27/SUN Fourier transform spectrometer (FTS) and MAX-DOAS in urban Beijing.