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Hyperbolic metamaterials are a class of materials exhibiting anisotropic dielectric function owing to the morphology of the nanostructures. In these structures, one direction behaves as a metal, and the orthogonal direction behaves as a dielectric material. Applications include subdiffraction imaging and hyperlenses. However, key limiting factors include energy losses of noble metals and challenging fabrication methods. In this work, self-assembled plasmonic metamaterials consisting of anisotropic nanoalloy pillars embedded into the ZnO matrix are developed using a seed-layer approach. Alloys of Au<i>_x</i>Al_1−<i>x</i> or Au<i>_x</i>Cu_1−<i>x</i> are explored due to their lower losses and higher stability. Optical and microstructural properties were explored. The ZnO-Au<i>_x</i>Cu_1−<i>x</i> system demonstrated excellent epitaxial quality and optical properties compared with the ZnO-Au<i>_x</i>Al_1−<i>x</i> system. Both nanocomposite systems demonstrate plasmonic resonance, hyperbolic dispersion, low losses, and epsilon-near-zero permittivity, making them promising candidates towards direct photonic integration.