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Low-dimensional nanomaterials have attracted considerable attention for next-generation flexible energy devices owing to their excellent electrochemical properties and superior flexibility. Herein, uniform Tellurium nanotubes (Te NTs) were prepared through a facile hydrothermal method, and then a flexible and freestanding electrode was fabricated with Te NTs as active materials and a small amount of nanofibrillated celluloses (NFCs) as a flexible matrix through a vacuum filtration method without adding extra conductive carbon or a binder. The resulting Te-based electrode exhibits a high volumetric capacity of 1512 mAh cm⁻³ at 200 mA g⁻¹, and delivers admirable cyclic stability (capacity retention of 104% over 300 cycles) and excellent rate performance (833 mAh cm⁻³ at 1000 mA g⁻¹), which benefits from the unique structure and intrinsically superior conductivity of Te NTs. After bending 50 times, the Te-based electrode delivers a desirable volumetric capacity of 1117 mAh cm⁻³, and remains 93% of initial capacity after 100 cycles. The results imply that the Te-based electrode exhibits excellent electrochemical properties and superior flexibility simultaneously, which can serve as a potential candidate for the flexible lithium batteries.