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Abstract A hybrid system interacts with the discrete and continuous dynamics of a physical dynamical system. The notion of a hybrid system gives embedded control systems a great advantage. The Langevin differential equation can accurately depict many physical phenomena and help researchers effectively represent anomalous diffusion. This paper considers a fractional hybrid Langevin differential equation, including the ψ-Caputo fractional operator. Furthermore, some novel boundaries selected are considered to be a problem. We used the Schauder and Banach fixed-point theorems to prove the existence and uniqueness of solutions to the considered problem. Additionally, the Ulam-Hyer stability is evaluated. Finally, we present a representative example to verify the theoretical outcomes of our findings.