Isolated attosecond pulse generation in a semi-infinite gas cell driven by time-gated phase matching

oleh: Federico Vismarra, Marina Fernández-Galán, Daniele Mocci, Lorenzo Colaizzi, Víctor Wilfried Segundo, Roberto Boyero-García, Javier Serrano, Enrique Conejero-Jarque, Marta Pini, Lorenzo Mai, Yingxuan Wu, Hans Jakob Wörner, Elisa Appi, Cord L. Arnold, Maurizio Reduzzi, Matteo Lucchini, Julio San Román, Mauro Nisoli, Carlos Hernández-García, Rocío Borrego-Varillas

Format: Article
Diterbitkan: Nature Publishing Group 2024-08-01

Deskripsi

Abstract Isolated attosecond pulse (IAP) generation usually involves the use of short-medium gas cells operated at high pressures. In contrast, long-medium schemes at low pressures are commonly perceived as inherently unsuitable for IAP generation due to the nonlinear phenomena that challenge favourable phase-matching conditions. Here we provide clear experimental evidence on the generation of isolated extreme-ultraviolet attosecond pulses in a semi-infinite gas cell, demonstrating the use of extended-medium geometries for effective production of IAPs. To gain a deeper understanding we develop a simulation method for high-order harmonic generation (HHG), which combines nonlinear propagation with macroscopic HHG solving the 3D time-dependent Schrödinger equation at the single-atom level. Our simulations reveal that the nonlinear spatio-temporal reshaping of the driving field, observed in the experiment as a bright plasma channel, acts as a self-regulating mechanism boosting the phase-matching conditions for the generation of IAPs.