Fluorescence-detected two-quantum and one-quantum-two-quantum 2D electronic spectros-copy of Rhodamine 700

oleh: Müller Stefan, Draeger Simon, Klosterhalfen Niklas, Brixner Tobias

Format: Article
Diterbitkan: EDP Sciences 2019-01-01

Deskripsi

We demonstrate the simultaneous acquisition of three fourth-order nonlinear signal contributions using a shot-to-shot-modulating pulse shaper and fluorescence detection. Beside the 1Q photon echo, two different species of two-quantum contributions can be isolated without any background via phase cycling.