Ultrafast charge transfer dynamics in 2D covalent organic frameworks/Re-complex hybrid photocatalyst
oleh: Qinying Pan, Mohamed Abdellah, Yuehan Cao, Weihua Lin, Yang Liu, Jie Meng, Quan Zhou, Qian Zhao, Xiaomei Yan, Zonglong Li, Hao Cui, Huili Cao, Wenting Fang, David Ackland Tanner, Mahmoud Abdel-Hafiez, Ying Zhou, Tonu Pullerits, Sophie E. Canton, Hong Xu, Kaibo Zheng
| Format: | Article |
|---|---|
| Diterbitkan: | Nature Portfolio 2022-02-01 |
Deskripsi
Re complexes within covalent organic frameworks have emerged as promising photocatalysts for CO2 reduction. Here, authors identify a high-energy electron transfer pathway during CO2 reduction that results in longer-lived excited states than a low-energy electron transfer pathway.