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Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China
oleh: W. Xu, X. S. Luo, Y. P. Pan, L. Zhang, A. H. Tang, J. L. Shen, Y. Zhang, K. H. Li, Q. H. Wu, D. W. Yang, Y. Y. Zhang, J. Xue, W. Q. Li, Q. Q. Li, L. Tang, S. H. Lu, T. Liang, Y. A. Tong, P. Liu, Q. Zhang, Z. Q. Xiong, X. J. Shi, L. H. Wu, W. Q. Shi, K. Tian, X. H. Zhong, K. Shi, Q. Y. Tang, L. J. Zhang, J. L. Huang, C. E. He, F. H. Kuang, B. Zhu, H. Liu, X. Jin, Y. J. Xin, X. K. Shi, E. Z. Du, A. J. Dore, S. Tang, J. L. Collett Jr., K. Goulding, Y. X. Sun, J. Ren, F. S. Zhang, X. J. Liu
| Format: | Article |
|---|---|
| Diterbitkan: | Copernicus Publications 2015-11-01 |
Deskripsi
A Nationwide Nitrogen Deposition Monitoring Network (NNDMN) containing 43 monitoring sites was established in China to measure gaseous NH<sub>3</sub>, NO<sub>2</sub>, and HNO<sub>3</sub> and particulate NH<sub>4</sub><sup>+</sup> and NO<sub>3</sub><sup>−</sup> in air and/or precipitation from 2010 to 2014. Wet/bulk deposition fluxes of N<sub>r</sub> species were collected by precipitation gauge method and measured by continuous-flow analyzer; dry deposition fluxes were estimated using airborne concentration measurements and inferential models. Our observations reveal large spatial variations of atmospheric N<sub>r</sub> concentrations and dry and wet/bulk N<sub>r</sub> deposition. On a national basis, the annual average concentrations (1.3–47.0 μg N m<sup>−3</sup>) and dry plus wet/bulk deposition fluxes (2.9–83.3 kg N ha<sup>−1</sup> yr<sup>−1</sup>) of inorganic N<sub>r</sub> species are ranked by land use as urban > rural > background sites and by regions as north China > southeast China > southwest China > northeast China > northwest China > Tibetan Plateau, reflecting the impact of anthropogenic N<sub>r</sub> emission. Average dry and wet/bulk N deposition fluxes were 20.6 ± 11.2 (mean ± standard deviation) and 19.3 ± 9.2 kg N ha<sup>−1</sup> yr<sup>−1</sup> across China, with reduced N deposition dominating both dry and wet/bulk deposition. Our results suggest atmospheric dry N deposition is equally important to wet/bulk N deposition at the national scale. Therefore, both deposition forms should be included when considering the impacts of N deposition on environment and ecosystem health.