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Many-body recombination in photoexcited insulating cuprates
oleh: Derek G. Sahota, Ruixing Liang, M. Dion, Patrick Fournier, Hanna A. DÄ…bkowska, Graeme M. Luke, J. Steven Dodge
Format: | Article |
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Diterbitkan: | American Physical Society 2019-12-01 |
Deskripsi
We study the pump-probe response of three insulating cuprates and develop a model for its recombination kinetics. The dependence on time, fluence, and both pump and probe photon energies implies many-body recombination on femtosecond timescales, characterized by anomalously large trapping and Auger coefficients. The fluence dependence follows a universal form that includes a characteristic volume scale, which we associate with the holon-doublon excitation efficiency. This volume varies strongly with pump photon energy and peaks at nearly twice the charge-transfer energy, suggesting that the variation is caused by carrier multiplication through impact ionization.