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Noise mechanisms in quantum systems can be broadly characterized as either coherent (i.e., unitary) or incoherent. For a given fixed average error rate, coherent noise mechanisms will generally lead to a larger worst-case error than incoherent noise. We show that the coherence of a noise source can be quantified by the unitarity , which we relate to the average change in purity averaged over input pure states. We then show that the unitarity can be efficiently estimated using a protocol based on randomized benchmarking that is efficient and robust to state-preparation and measurement errors. We also show that the unitarity provides a lower bound on the optimal achievable gate infidelity under a given noisy process.