Interfacial Electronic Modulation of Dual-Monodispersed Pt–Ni3S2 as Efficacious Bi-Functional Electrocatalysts for Concurrent H2 Evolution and Methanol Selective Oxidation
oleh: Qianqian Zhao, Bin Zhao, Xin Long, Renfei Feng, Mohsen Shakouri, Alisa Paterson, Qunfeng Xiao, Yu Zhang, Xian-Zhu Fu, Jing-Li Luo
| Format: | Article |
|---|---|
| Diterbitkan: | SpringerOpen 2024-01-01 |
Deskripsi
Highlights The well-conceived Pt–Ni3S2 heteronanocrystals with dual-monodispersed characteristics are synthesized through interfacial electronic modulation. The asymmetrical charge distribution at Pt–Ni3S2 hetero-interface results in the formation of high-valent Ni sites and negatively-charged Pt δ−. It eventually accelerates water dissociation and achieves the steady concurrent generation of value-added formate and hydrogen.