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Softening of a flat phonon mode in the kagome ScV6Sn6
oleh: A. Korshunov, H. Hu, D. Subires, Y. Jiang, D. Călugăru, X. Feng, A. Rajapitamahuni, C. Yi, S. Roychowdhury, M. G. Vergniory, J. Strempfer, C. Shekhar, E. Vescovo, D. Chernyshov, A. H. Said, A. Bosak, C. Felser, B. Andrei Bernevig, S. Blanco-Canosa
Format: | Article |
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Diterbitkan: | Nature Portfolio 2023-10-01 |
Deskripsi
Abstract Geometrically frustrated kagome lattices are raising as novel platforms to engineer correlated topological electron flat bands that are prominent to electronic instabilities. Here, we demonstrate a phonon softening at the k z = π plane in ScV6Sn6. The low energy longitudinal phonon collapses at ~98 K and q = $$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$ 1 3 1 3 1 2 due to the electron-phonon interaction, without the emergence of long-range charge order which sets in at a different propagation vector q CDW = $$\frac{1}{3}\frac{1}{3}\frac{1}{3}$$ 1 3 1 3 1 3 . Theoretical calculations corroborate the experimental finding to indicate that the leading instability is located at $$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$ 1 3 1 3 1 2 of a rather flat mode. We relate the phonon renormalization to the orbital-resolved susceptibility of the trigonal Sn atoms and explain the approximately flat phonon dispersion. Our data report the first example of the collapse of a kagome bosonic mode and promote the 166 compounds of kagomes as primary candidates to explore correlated flat phonon-topological flat electron physics.