Rapid multiple-quantum three-dimensional fluorescence spectroscopy disentangles quantum pathways

oleh: Stefan Mueller, Julian Lüttig, Pavel Malý, Lei Ji, Jie Han, Michael Moos, Todd B. Marder, Uwe H. F. Bunz, Andreas Dreuw, Christoph Lambert, Tobias Brixner

Format: Article
Diterbitkan: Nature Portfolio 2019-10-01

Deskripsi

Multidimensional spectroscopic tools are important to explore the details of molecular dynamics. Here the authors use shaped pulses to demonstrate a 3D fluorescence spectroscopy method to extract the fourth and higher-order nonlinear responses in light-molecule interaction.