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The title compound, [ZnBr2(C11H13N3)], was synthesized by hydrothermal reaction of ZnBr2 and (S)-2-(pyrrolidin-2-yl)-1H-benzimidazole. The ZnII atom has a distorted tetrahedral geometry and is coordinated by two N atoms from the chelating organic ligand and two terminal Br− anions. In the crystal structure, molecules are linked into a chain along the [101] direction by N—H...Br and C—H...Br hydrogen bonds.