Dzyaloshinsky–Moriya Interaction Induced Anomalous <i>g</i> Behavior of Sr<sub>2</sub>IrO<sub>4</sub> Probed by Electron Spin Resonance

oleh: Kai Wang, Liqin Yan, Youguo Shi, Baogen Shen, Lunhua He, Fangwei Wang, Jun Lu, Tongyun Zhao, Zunming Lu

Format: Article
Diterbitkan: MDPI AG 2023-11-01

Deskripsi

Among the 5d transition metal iridates, Sr<sub>2</sub>IrO<sub>4</sub>, which has a layered chalcogenide structure, has received much attention due to its strong spin–orbit coupling (SOC), which produces Mott insulating states and anomalous physical behaviors. In this paper, the microscopic magnetism of Sr<sub>2</sub>IrO<sub>4</sub> is studied with electron spin resonance (ESR) measurements. The Lande factor <i>g</i> of the ferromagnetic resonance signal of Sr<sub>2</sub>IrO<sub>4</sub> shows anomalous behavior compared to typical ferromagnets. It gradually decreases, and the corresponding resonance field <i>H</i><sub>r</sub> increases, with decreasing temperature. The various physical parameters. including the saturated magnetic field <i>H</i><sub>s</sub> derived from <i>M-H</i>, <i>H</i><sub>r</sub>, Δ<i>H</i><sub>pp</sub>, the <i>g</i> factor and the intensity <i>I</i> extracted from ESR spectra, are analyzed in detail. Eventually, it is revealed that the anomalous behavior of the <i>g</i>-factor is induced by in-plane Dzyaloshinsky–Moriya interaction (DMI) rather than the SOC effect.