Coordination environment dependent selectivity of single-site-Cu enriched crystalline porous catalysts in CO2 reduction to CH4

oleh: Yu Zhang, Long-Zhang Dong, Shan Li, Xin Huang, Jia-Nan Chang, Jian-Hui Wang, Jie Zhou, Shun-Li Li, Ya-Qian Lan

Format: Article
Diterbitkan: Nature Portfolio 2021-11-01

Deskripsi

Crystalline porous catalysts with single Cu sites are dedicated to exploring the dependence of CO2 electroreduction selectivity on the coordination environment of catalytic sites. The conductive MOF Cu-DBC with oxygen-coordinated Cu sites shows a high Faradaic efficiency ~80% of CO2-to-CH4.