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This paper presents a novel calibration method for micro-electro mechanical system gyroscope in attitude measurement system of small rotor unmanned aerial vehicles. This method is based on an observation vector and its cross product, which is especially valuable for the in-field calibration without the aid of external equipment. By analysing the error model of the tri-axial gyroscope, the principle of calibration is proposed. Compared with other algorithms, numerical simulations are performed to evaluate the effectiveness of integral form of the cross product calibration method. Experiment on the hex-rotor unmanned aerial vehicle platform shows that the proposed method has great advantages in low-cost integrated navigation system.