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Abstract We present the result of the quadratic-in-spin interaction Hamiltonian for binary systems of rotating compact objects with generic spins, up to N3LO corrections within the post-Newtonian expansion. The calculation is performed by employing the effective field theory diagrammatic approach, and it involves Feynman integrals up to three loops, evaluated within the dimensional regularization scheme. The gauge-invariant binding energy and the scattering angle, in special kinematic regimes and spin configurations, are explicitly derived. The results extend our earlier study on the spin-orbit interaction effects.