Why is the Indo-Gangetic Plain the region with the largest NH<sub>3</sub> column in the globe during pre-monsoon and monsoon seasons?

oleh: T. Wang, Y. Song, Z. Xu, M. Liu, T. Xu, T. Xu, W. Liao, L. Yin, X. Cai, L. Kang, H. Zhang, T. Zhu, T. Zhu

Format: Article
Diterbitkan: Copernicus Publications 2020-07-01

Deskripsi

<p>Satellite observations show a global maximum in ammonia (<span class="inline-formula">NH<sub>3</sub></span>) over the Indo-Gangetic Plain (IGP), with a peak from June to August. However, it has never been explained explicitly. In this study, we investigated the causes of high <span class="inline-formula">NH<sub>3</sub></span> loading over the IGP during the pre-monsoon and monsoon seasons using WRF-Chem (Weather Research and Forecasting model coupled to chemistry). The IGP has relatively high <span class="inline-formula">NH<sub>3</sub></span> emission fluxes (0.4&thinsp;t&thinsp;km<span class="inline-formula"><sup>−2</sup></span>&thinsp;month<span class="inline-formula"><sup>−1</sup>)</span> due to intensive agricultural activities and high air temperature from June to August. Additionally, low sulfur dioxide (<span class="inline-formula">SO<sub>2</sub></span>) and nitrogen oxides (<span class="inline-formula">NO<sub><i>x</i></sub></span>) emissions and high air temperature limit the gas-to-particle conversion of <span class="inline-formula">NH<sub>3</sub></span>, particularly for ammonium nitrate formation. Moreover, the barrier effects of the Himalayas in combination with the surface convergence weaken the horizontal diffusion of <span class="inline-formula">NH<sub>3</sub></span>. The high <span class="inline-formula">NH<sub>3</sub></span> loading over the IGP mainly results from the low gas-to-particle partitioning of <span class="inline-formula">NH<sub>3</sub></span> caused by low <span class="inline-formula">SO<sub>2</sub></span> and <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions. It contrasts to those in the North China Plain, where high <span class="inline-formula">SO<sub>2</sub></span> and <span class="inline-formula">NO<sub><i>x</i></sub></span> emissions promote the conversion of gaseous <span class="inline-formula">NH<sub>3</sub></span> into particulate ammonium.</p>