Global impact of the COVID-19 lockdown on surface concentration and health risk of atmospheric benzene
oleh: C. Ling, L. Cui, R. Li, R. Li
| Format: | Article |
|---|---|
| Diterbitkan: | Copernicus Publications 2023-03-01 |
Deskripsi
<p>To curb the spread of the COVID-19 pandemic, many countries around the world imposed an unprecedented lockdown, producing reductions in pollutant emissions. Unfortunately, the lockdown-driven global ambient benzene changes still remain unknown. An ensemble machine-learning model coupled with chemical transport models (CTMs) was applied to estimate global high-resolution ambient benzene levels. Afterwards, the extreme gradient boosting (XGBoost) algorithm was employed to decouple the contributions of meteorology and emission reduction to ambient benzene. The change ratio (<span class="inline-formula"><i>P</i><sub>dew</sub></span>) of the deweathered benzene concentration from the pre-lockdown to lockdown period was in the order of India (<span class="inline-formula">−23.6</span> %) <span class="inline-formula">></span> Europe (<span class="inline-formula">−21.9</span> %) <span class="inline-formula">></span> the United States (<span class="inline-formula">−16.2</span> %) <span class="inline-formula">></span> China (<span class="inline-formula">−15.6</span> %). The detrended change (<span class="inline-formula"><i>P</i><sup>∗</sup></span>) of the deweathered benzene level (change ratio in 2020 <span class="inline-formula">−</span> change ratio in 2019) followed the order of India (<span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M11" display="inline" overflow="scroll" dspmath="mathml"><mrow><msup><mi>P</mi><mo>*</mo></msup><mo>=</mo><mo>-</mo><mn mathvariant="normal">16.2</mn></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="55pt" height="11pt" class="svg-formula" dspmath="mathimg" md5hash="852b46592b1dfc654f40713391ad0a3e"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00001.svg" width="55pt" height="11pt" src="acp-23-3311-2023-ie00001.png"/></svg:svg></span></span> %) <span class="inline-formula">></span> Europe (<span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M13" display="inline" overflow="scroll" dspmath="mathml"><mrow><msup><mi>P</mi><mo>∗</mo></msup><mo>=</mo><mo>-</mo><mn mathvariant="normal">13.9</mn></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="55pt" height="11pt" class="svg-formula" dspmath="mathimg" md5hash="712abd5f6894974ee3da4a2af6e00f96"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00002.svg" width="55pt" height="11pt" src="acp-23-3311-2023-ie00002.png"/></svg:svg></span></span> %) <span class="inline-formula">></span> China (<span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M15" display="inline" overflow="scroll" dspmath="mathml"><mrow><msup><mi>P</mi><mo>∗</mo></msup><mo>=</mo><mo>-</mo><mn mathvariant="normal">13.3</mn></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="55pt" height="11pt" class="svg-formula" dspmath="mathimg" md5hash="baa35aa5281d9a0ef24f77a794a21914"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00003.svg" width="55pt" height="11pt" src="acp-23-3311-2023-ie00003.png"/></svg:svg></span></span> %) <span class="inline-formula">></span> the United States (<span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M17" display="inline" overflow="scroll" dspmath="mathml"><mrow><msup><mi>P</mi><mo>∗</mo></msup><mo>=</mo><mo>-</mo><mn mathvariant="normal">6.00</mn></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="55pt" height="11pt" class="svg-formula" dspmath="mathimg" md5hash="3c55c747468e9828db95e0548fd42fb3"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00004.svg" width="55pt" height="11pt" src="acp-23-3311-2023-ie00004.png"/></svg:svg></span></span> %). Emission reductions derived from industrial activities and transportation were major drivers for the benzene decrease during the lockdown period. The highest decreasing ratio of ambient benzene in India might be associated with local serious benzene pollution during the business-as-usual period and restricted transportation after lockdown. Substantial decreases in atmospheric benzene levels had significant health benefits. The global average lifetime carcinogenic risk (LCR) and hazard index (HI) decreased from <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M18" display="inline" overflow="scroll" dspmath="mathml"><mrow><mn mathvariant="normal">4.89</mn><mo>×</mo><msup><mn mathvariant="normal">10</mn><mrow><mo>-</mo><mn mathvariant="normal">7</mn></mrow></msup></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="57pt" height="13pt" class="svg-formula" dspmath="mathimg" md5hash="fc272dc0e404943d6a129e31f6fe91f8"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00005.svg" width="57pt" height="13pt" src="acp-23-3311-2023-ie00005.png"/></svg:svg></span></span> and <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M19" display="inline" overflow="scroll" dspmath="mathml"><mrow><mn mathvariant="normal">5.90</mn><mo>×</mo><msup><mn mathvariant="normal">10</mn><mrow><mo>-</mo><mn mathvariant="normal">3</mn></mrow></msup></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="57pt" height="14pt" class="svg-formula" dspmath="mathimg" md5hash="e50515613afb64ee7d8c917f5100d8a5"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00006.svg" width="57pt" height="14pt" src="acp-23-3311-2023-ie00006.png"/></svg:svg></span></span> to <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M20" display="inline" overflow="scroll" dspmath="mathml"><mrow><mn mathvariant="normal">4.51</mn><mo>×</mo><msup><mn mathvariant="normal">10</mn><mrow><mo>-</mo><mn mathvariant="normal">7</mn></mrow></msup></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="57pt" height="13pt" class="svg-formula" dspmath="mathimg" md5hash="6c435be40f9e808ec2df6e4de9993193"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00007.svg" width="57pt" height="13pt" src="acp-23-3311-2023-ie00007.png"/></svg:svg></span></span> and <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M21" display="inline" overflow="scroll" dspmath="mathml"><mrow><mn mathvariant="normal">5.40</mn><mo>×</mo><msup><mn mathvariant="normal">10</mn><mrow><mo>-</mo><mn mathvariant="normal">3</mn></mrow></msup></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="57pt" height="14pt" class="svg-formula" dspmath="mathimg" md5hash="d9b5ca6615ed0a40d7512e2392edd98c"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-23-3311-2023-ie00008.svg" width="57pt" height="14pt" src="acp-23-3311-2023-ie00008.png"/></svg:svg></span></span>, respectively. China and India showed higher health benefits due to benzene pollution mitigation compared with other countries, highlighting the importance of benzene emission reduction.</p>