Characteristics of Coherent Optical Phonons in a Hexagonal YMnO<sub>3</sub> Thin Film

oleh: Takayuki Hasegawa

Format: Article
Diterbitkan: MDPI AG 2019-02-01

Deskripsi

This paper reviews our recent study on a coherent optical phonon in a hexagonal YMnO<sub>3</sub> thin film together with related optical studies in hexagonal <i>R</i>MnO<sub>3</sub> (<i>R</i> = Y, Lu, Ho) compounds. Coherent phonons have been observed in <i>R</i>MnO<sub>3</sub> compounds by pump-probe spectroscopy with subpicosecond laser pulses, whereas the observation of coherent optical phonons was reported only in LuMnO<sub>3</sub>. Recently, we succeeded in the observation of the coherent optical phonon in a YMnO<sub>3</sub> thin film. The generation process of the coherent optical phonon is assigned to a displacive mechanism, which is identical to that in LuMnO<sub>3</sub>. The coherent optical phonon is observed in the temperature range from 10 K to room temperature, while the oscillation intensity strongly decreases as the temperature increases to the N&#233;el temperature of ~70 K from a lower temperature range. It is interesting that the temperature dependence is largely different from that in LuMnO<sub>3</sub>. We describe that the result can be qualitatively explained by the property of an isostructural transition around the N&#233;el temperature in <i>R</i>MnO<sub>3</sub> compounds. In addition, we briefly discuss ultrafast incoherent responses of excited electronic states from the viewpoint of the excitation photon energy of laser pulses.