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The main concern of this manuscript is to study the optimal control problem for Hilfer fractional neutral stochastic integrodifferential systems with infinite delay. Initially, we establish the existence of mild solutions for the Hilfer fractional stochastic integrodifferential system with infinite delay via applying fractional calculus, semigroups, stochastic analysis techniques, and the Banach fixed point theorem. In addition, we establish the existence of mild solutions of the Hilfer fractional neutral stochastic delay integrodifferential system. Further, we investigate the existence of optimal pairs for the Hilfer fractional neutral stochastic delay integrodifferential systems. We provide an illustration to clarify our results.