NO<sub><i>x</i></sub> lifetimes and emissions of cities and power plants in polluted background estimated by satellite observations

oleh: F. Liu, F. Liu, F. Liu, S. Beirle, Q. Zhang, S. Dörner, K. He, K. He, T. Wagner

Format: Article
Diterbitkan: Copernicus Publications 2016-04-01

Deskripsi

We present a new method to quantify NO<sub><i>x</i></sub> emissions and corresponding atmospheric lifetimes from OMI NO<sub>2</sub> observations together with ECMWF wind fields without further model input for sources located in a polluted background. NO<sub>2</sub> patterns under calm wind conditions are used as proxy for the spatial patterns of NO<sub><i>x</i></sub> emissions, and the effective atmospheric NO<sub><i>x</i></sub> lifetime is determined from the change of spatial patterns measured at larger wind speeds. Emissions are subsequently derived from the NO<sub>2</sub> mass above the background, integrated around the source of interest. <br><br> Lifetimes and emissions are estimated for 17 power plants and 53 cities located in non-mountainous regions across China and the USA. The derived lifetimes for the ozone season (May–September) are 3.8 ± 1.0 h (mean ± standard deviation) with a range of 1.8 to 7.5 h. The derived NO<sub><i>x</i></sub> emissions show generally good agreement with bottom-up inventories for power plants and cities. Regional inventory shows better agreement with top-down estimates for Chinese cities compared to global inventory, most likely due to different downscaling approaches adopted in the two inventories.