Strong optical response and light emission from a monolayer molecular crystal

oleh: Huijuan Zhao, Yingbo Zhao, Yinxuan Song, Ming Zhou, Wei Lv, Liu Tao, Yuzhang Feng, Biying Song, Yue Ma, Junqing Zhang, Jun Xiao, Ying Wang, Der-Hsien Lien, Matin Amani, Hyungjin Kim, Xiaoqing Chen, Zhangting Wu, Zhenhua Ni, Peng Wang, Yi Shi, Haibo Ma, Xiang Zhang, Jian-Bin Xu, Alessandro Troisi, Ali Javey, Xinran Wang

Format: Article
Diterbitkan: Nature Portfolio 2019-12-01

Deskripsi

The optical response of inorganic two-dimensional semiconductors is dominated by Wannier-Mott excitons, but molecular systems can host localised Frenkel excitons. Here, the authors report strong optical response in a class of monolayer molecular J-aggregates due to the coherent Coulomb interaction between localised Frenkel excitons.