Measurement of transient strain induced by two-photon excitation

oleh: S. P. Zeuschner, J.-E. Pudell, A. von Reppert, M. Deb, E. Popova, N. Keller, M. Rössle, M. Herzog, M. Bargheer

Format: Article
Diterbitkan: American Physical Society 2020-04-01

Deskripsi

By ultrafast x-ray diffraction we quantify the strain from coherent and incoherent phonons generated by one- and two-photon absorption. We investigated the ferrimagnetic insulator bismuth-doped yttrium iron garnet, which is a workhorse for laser-induced spin dynamics that may be excited indirectly via phonons. We identify the two-photon absorption by the quadratic intensity dependence of the transient strain and confirm a short lifetime of the intermediate state via the inverse proportional dependence on the pump-pulse duration. We determine the two-photon absorption coefficient using the linear relation between strain and absorbed energy density. For large intensities of about 1TW/cm^{2} considerable strain amplitudes of 0.1% are driven exclusively by two-photon absorption.