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One of the advantages of multimedia-assisted instruction is that it makes students more interested in sustainable learning and assists them to access information and learn more effectively. This research sought to explore the asymmetric effects of the development of sustainable multimedia-assisted instruction (MAI) on student reading practice in areas such as the implementation of learner autonomy and the improvement of reading ability, primarily based on multimedia technology-assisted instruction. This experiment was conducted in a junior high school in China. Eighty-six students from two parallel grade two classes were selected as research participants. Class One was set as the experimental class (EC) and Class Two was symmetrically designed as the control class (CC). The research results indicate that MAI encouraged students in the EC to adopt reading strategies more frequently and helped them to improve their level of learner autonomy, from a low level to an intermediate level, for the use of an asymmetrical technology, in comparison with the control class. Furthermore, the EC’s reading ability was significantly enhanced. Additionally, there is a discussion of pedagogical implications and constructive suggestions considered to be beneficial for sustainable learning skills, teaching and for further research on the symmetrical application of technology in education. Finally, one of the most significant findings from this study is the effectiveness of combining modern sustainable technology and advanced educational concepts with symmetry in promoting learner autonomy within a sustainable learning model.