Voltage control of magnetism in Fe3-x GeTe2/In2Se3 van der Waals ferromagnetic/ferroelectric heterostructures

oleh: Jaeun Eom, In Hak Lee, Jung Yun Kee, Minhyun Cho, Jeongdae Seo, Hoyoung Suh, Hyung-Jin Choi, Yumin Sim, Shuzhang Chen, Hye Jung Chang, Seung-Hyub Baek, Cedomir Petrovic, Hyejin Ryu, Chaun Jang, Young Duck Kim, Chan-Ho Yang, Maeng-Je Seong, Jin Hong Lee, Se Young Park, Jun Woo Choi

Format: Article
Diterbitkan: Nature Portfolio 2023-09-01

Deskripsi

Abstract We investigate the voltage control of magnetism in a van der Waals (vdW) heterostructure device consisting of two distinct vdW materials, the ferromagnetic Fe3-x GeTe2 and the ferroelectric In2Se3. It is observed that gate voltages applied to the Fe3-x GeTe2/In2Se3 heterostructure device modulate the magnetic properties of Fe3-x GeTe2 with significant decrease in coercive field for both positive and negative voltages. Raman spectroscopy on the heterostructure device shows voltage-dependent increase in the in-plane In2Se3 and Fe3-x GeTe2 lattice constants for both voltage polarities. Thus, the voltage-dependent decrease in the Fe3-x GeTe2 coercive field, regardless of the gate voltage polarity, can be attributed to the presence of in-plane tensile strain. This is supported by density functional theory calculations showing tensile-strain-induced reduction of the magnetocrystalline anisotropy, which in turn decreases the coercive field. Our results demonstrate an effective method to realize low-power voltage-controlled vdW spintronic devices utilizing the magnetoelectric effect in vdW ferromagnetic/ferroelectric heterostructures.