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Abstract Identifying pigments from colored relics is essential for their color restoration and for facsimile creation. A workflow for identifying pigment information is constructed based on visible spectral imaging technology, aligned with the drawing process of colored relics. This workflow includes three steps: boundary extraction, material identification and prediction of mixture proportions. The methods for segmenting visible spectral images, identifying chemical compositions, and predicting mixture proportions of pigments are extensively reviewed. Future research trends of these methods are also analyzed. The influence of the pigment particle size is currently underexplored but can be accomplished by multidisciplinary research.