High-order harmonic generation from hybrid organic–inorganic perovskite thin films
oleh: Hideki Hirori, Peiyu Xia, Yasushi Shinohara, Tomohito Otobe, Yasuyuki Sanari, Hirokazu Tahara, Nobuhisa Ishii, Jiro Itatani, Kenichi L. Ishikawa, Tomoko Aharen, Masashi Ozaki, Atsushi Wakamiya, Yoshihiko Kanemitsu
| Format: | Article |
|---|---|
| Diterbitkan: | AIP Publishing LLC 2019-04-01 |
Deskripsi
The generation of high-order harmonics from hybrid organic–inorganic perovskites (HOIPs) is demonstrated by the excitation with a strong mid-infrared laser pulse. We prepare three types of HOIP polycrystalline thin film samples by solution processes (MAPbX3; MA = CH3NH3+; X = I, Br, Cl). The high-order harmonics from the sample (MAPbBr3) are more than tenfold stronger than those from the well-studied GaSe crystal despite their comparable bandgap energies, implying that the stronger band-to-band transition of the HOIPs causes the higher yields.