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Rational design of carbon nitride photocatalysts by identification of cyanamide defects as catalytically relevant sites
oleh: Vincent Wing-hei Lau, Igor Moudrakovski, Tiago Botari, Simon Weinberger, Maria B. Mesch, Viola Duppel, Jürgen Senker, Volker Blum, Bettina V. Lotsch
Format: | Article |
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Diterbitkan: | Nature Portfolio 2016-07-01 |
Deskripsi
Graphitic carbon nitride is a promising hydrogen evolution photocatalyst, although there is limited understanding of its mechanistic operation. Here, the authors employ molecular heptazine-based model catalysts to identify catalytically relevant defects and to rationally design a highly active carbon nitride photocatalyst.