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Plasmonically Enhanced Colloidal Quantum Dot/Graphene Doped Polymer Random Lasers
oleh: Mingxuan Cao, Min Wang, Zhiwen Wang, Luhao Zang, Hao Liu, Shuping Xiao, Matthew M. F. Yuen, Ying Wang, Yating Zhang, Jianquan Yao
Format: | Article |
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Diterbitkan: | MDPI AG 2022-03-01 |
Deskripsi
An improvement in random lasers based on a colloidal quantum dot (QD)/graphene-doped polymer was observed and attributed to multiple light-scattering and graphene surface plasmon resonance. The emission characteristics of quantum dots doped with graphene oxide and reduced graphene oxide were compared. The QD/reduced graphene oxide hybrid exhibited a lower laser emission threshold (~460 μJ/cm<sup>2</sup>). The emission modes and thresholds were strongly dependent on both the graphene doping concentration and the external temperature. Decreased plasmon coupling was the primary reason for lower QD/graphene laser emission with increasing temperature. The optimum reduced graphene oxide concentration was 0.2 wt.%. This work provides a practical approach to optimizing the threshold and stability of random laser devices, with potential applications in displays, sensors, and anti-counterfeiting labels.